Hermitage, S. and Howard, J. A. K. and Jay, D. and Pritchard, R. G. and Probert, M. R. and Whiting, A. (2004) 'Mechanistic studies on the formal aza-Diels-Alder reactions of N-aryl imines : evidence for the non-concertedness under Lewis-acid catalysed conditions.', Organic & biomolecular chemistry., 2 (17). pp. 2451-2460.
The reaction of a para-methoxyaniline, ethyl glyoxalate-derived imine with a series of dienes has resulted in products, which initially suggest the operation of different modes of aza-Diels-Alder reaction. However, a more likely explanation is that a common reaction mechanism is operating, involving a step-wise Lewis-acid catalysed process, which only appears to behave similarly to alternative concerted cycloaddition reactions.
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|Publisher Web site:||http://dx.doi.org/10.1039/B407293F|
|Record Created:||03 May 2007|
|Last Modified:||08 Apr 2009 16:31|
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