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Low-temperature interactions of magnetic excitons in LaCoO(3).

Giblin, S.R. and Terry, I. and Prabhakaran, D. and Boothroyd, A.T. and Leighton, C. (2009) 'Low-temperature interactions of magnetic excitons in LaCoO(3).', Physical review B., 79 (17). p. 174410.

Abstract

The low-temperature magnetic behavior of LaCoO3, containing oxygen vacancies, is reported. Magnetic-susceptibility measurements made in the temperature range of 0.5–35 K on a single crystal and a polycrystalline sample provide strong evidence for the existence of magnetic excitons as fundamental entities within the bulk of the material system. Specifically, two distinct types of excitons form, isolated and interacting excitons, both of which are associated with oxygen vacancies. Isolated magnetic excitons act as high-spin paramagnetic particles while the interacting excitons appear to be coupled antiferromagnetically. It is proposed that the interaction arises from the overlap of magnetic excitons as a consequence of the statistical clustering of oxygen vacancies. The striking similarity of these results with those of the lightly doped La0.97Sr0.03CoO3 suggests that the observed excitons are a precursor to magneto-electronic phase separation and supports the idea that phase separation is initiated by disorder in the material system.

Item Type:Article
Full text:PDF - Published Version (171Kb)
Status:Peer-reviewed
Publisher Web site:http://dx.doi.org/10.1103/PhysRevB.79.174410
Record Created:12 Aug 2011 11:05
Last Modified:18 Aug 2011 16:15

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