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Role of Nonvalence States in the Ultrafast Dynamics of Isolated Anions

Verlet, Jan R.R.; Anstöter, Cate S.; Bull, James N.; Rogers, Joshua P.

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Authors

Cate S. Anstöter

James N. Bull

Joshua P. Rogers



Abstract

Nonvalence states of neutral molecules (Rydberg states) play important roles in nonadiabatic dynamics of excited states. In anions, such nonadiabatic transitions between nonvalence and valence states have been much less explored even though they are believed to play important roles in electron capture and excited state dynamics of anions. The aim of this Feature Article is to provide an overview of recent experimental observations, based on time-resolved photoelectron imaging, of valence to nonvalence and nonvalence to valence transitions in anions and to demonstrate that such dynamics may be commonplace in the excited state dynamics of molecular anions and cluster anions.

Citation

Verlet, J. R., Anstöter, C. S., Bull, J. N., & Rogers, J. P. (2020). Role of Nonvalence States in the Ultrafast Dynamics of Isolated Anions. The Journal of Physical Chemistry A, 124(18), 3507-3519. https://doi.org/10.1021/acs.jpca.0c01260

Journal Article Type Article
Online Publication Date Apr 1, 2020
Publication Date May 7, 2020
Deposit Date May 13, 2020
Publicly Available Date Mar 29, 2024
Journal The Journal of Physical Chemistry A
Print ISSN 1089-5639
Electronic ISSN 1520-5215
Publisher American Chemical Society
Peer Reviewed Peer Reviewed
Volume 124
Issue 18
Pages 3507-3519
DOI https://doi.org/10.1021/acs.jpca.0c01260

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Copyright Statement
This is an open access article published under an ACS AuthorChoice License, which permits copying and redistribution of the article or any adaptations for non-commercial purposes.




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